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020 ▼a 9781687931672
035 ▼a (MiAaPQ)AAI13900305
040 ▼a MiAaPQ ▼c MiAaPQ ▼d 247004
0820 ▼a 530
1001 ▼a Zhang, Jiawei.
24510 ▼a Infrared and Terahertz Near-field Spectroscopy and Microscopy on 3d and 4d Correlated Electron Materials.
260 ▼a [S.l.]: ▼b State University of New York at Stony Brook., ▼c 2019.
260 1 ▼a Ann Arbor: ▼b ProQuest Dissertations & Theses, ▼c 2019.
300 ▼a 105 p.
500 ▼a Source: Dissertations Abstracts International, Volume: 81-05, Section: B.
500 ▼a Advisor: Liu, Mengkun.
5021 ▼a Thesis (Ph.D.)--State University of New York at Stony Brook, 2019.
506 ▼a This item must not be sold to any third party vendors.
520 ▼a The electromagnetic waves in the far infrared and terahertz range have ubiquitous applications to the optical characterization of solid-state materials in which numerous physical phenomena occur within the energy range below ~ 100 meV ( molecular rotation, exciton transition, superconducting gap opening, etc.). Conventional infrared and terahertz characterization methods have been suffering from low spatial resolution due to optical diffraction effects. This thesis presents a new type of micro-imaging technique named scattering-type scanning near-field optical microscopy (s-SNOM) which can reach deep subwavelength spatial resolution regardless of the wavelength of probing light. The working principle of far infrared s-SNOM is introduced with an illustration of two experimental measurements on the insulator-to-metal phase transition (IMT) of transition metal oxides Ca2RuO4 and VO2, the images of phase boundaries on sample surfaces show exotic nanoscale phase patterns, revealing the competition between strain and domain wall energy, showing the complex interplay between non-equilibrium electronic and lattice steady states. The second part of the thesis discusses the terahertz time domain spectroscopy (THz-TDS) and optical-pump-terahertz-probe (OPTP) schemes. An experiment is demonstrated to explore the ultrafast electronic dynamics of correlated electron materials V1-xNbxO2 thin films, revealing a novel way of tuning electron-electron and electron-phonon interaction dynamics. The last part of the thesis reports our recent progress in THz s-SNOM with a demonstration of near field imaging on graphene. Measurement suggests that a single layer graphene acts as a perfect terahertz reflector in the near-field regime due to high-momentum effects. Conclusions and potential works for the future are mentioned at last.
590 ▼a School code: 0771.
650 4 ▼a Physics.
690 ▼a 0605
71020 ▼a State University of New York at Stony Brook. ▼b Physics.
7730 ▼t Dissertations Abstracts International ▼g 81-05B.
773 ▼t Dissertation Abstract International
790 ▼a 0771
791 ▼a Ph.D.
792 ▼a 2019
793 ▼a English
85640 ▼u http://www.riss.kr/pdu/ddodLink.do?id=T15492169 ▼n KERIS ▼z 이 자료의 원문은 한국교육학술정보원에서 제공합니다.
980 ▼a 202002 ▼f 2020
990 ▼a ***1008102
991 ▼a E-BOOK