자료유형 | 학위논문 |
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서명/저자사항 | Chemical Thermodynamics of Water Soluble Organic Compounds Found in Aqueous Atmospheric Aerosols: Modeling and Microfluidic Measurements. |
개인저자 | Nandy, Lucy. |
단체저자명 | University of Minnesota. Mechanical Engineering. |
발행사항 | [S.l.]: University of Minnesota., 2018. |
발행사항 | Ann Arbor: ProQuest Dissertations & Theses, 2018. |
형태사항 | 334 p. |
기본자료 저록 | Dissertation Abstracts International 80-01B(E). Dissertation Abstract International |
ISBN | 9780438351349 |
학위논문주기 | Thesis (Ph.D.)--University of Minnesota, 2018. |
일반주기 |
Source: Dissertation Abstracts International, Volume: 80-01(E), Section: B.
Adviser: Cari S. Dutcher. |
요약 | Atmospheric aerosols, suspensions of tiny particulates in atmosphere, are known to have a major impact on Earth's climate. Due to the highly chemically and physically complex nature of aerosol particles, large uncertainty in climate modeling ari |
요약 | The specific objectives attained in this dissertation research are as follows. |
요약 | I. Aqueous Solution Thermodynamic Model Development: Thermodynamic analytic predictive models using statistical mechanics were developed for multicomponent systems across the entire range of equilibrium relative humidity (RH - 0 to 100%). The mo |
요약 | II. Model Applications: (1) pH of aerosols was evaluated in a collaborative work, which is of significant interest due to its effect on the environment. (2) Hygroscopicity was estimated in a collaborative work, which has effects on the optical p |
요약 | III. Experimental Microfluidics: The thermodynamic model was parameterized and validated with measurements of water uptake of multicomponent aerosol particles. The influence of relative humidity on phase behavior to assess the effects on water l |
요약 | The efforts in this dissertation together will enhance understanding of atmospheric aerosol phase, solid/liquid/gas partitioning, and liquid-liquid morphologies found in the troposphere. Additionally, the measurements and modeling performed here |
일반주제명 | Mechanical engineering. Atmospheric chemistry. Chemical engineering. |
언어 | 영어 |
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