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Advancing Frontiers in Reactive and Selective Iridium C-H Borylation Catalysis and Targeted Silsesquioxane Synthesis

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서명/저자사항Advancing Frontiers in Reactive and Selective Iridium C-H Borylation Catalysis and Targeted Silsesquioxane Synthesis.
개인저자Dannatt, Jonathan E.
단체저자명Michigan State University. Chemistry - Doctor of Philosophy.
발행사항[S.l.]: Michigan State University., 2019.
발행사항Ann Arbor: ProQuest Dissertations & Theses, 2019.
형태사항521 p.
기본자료 저록Dissertations Abstracts International 81-03B.
Dissertation Abstract International
ISBN9781085673259
학위논문주기Thesis (Ph.D.)--Michigan State University, 2019.
일반주기 Source: Dissertations Abstracts International, Volume: 81-03, Section: B.
Advisor: Maleczka, Rob.
이용제한사항This item must not be sold to any third party vendors.
요약The studies in this dissertation are aimed at uncovering reactive and selective Ir-catalyzed C-H borylation (CHB) catalysts. Due to the high versatility of organoboron species, green methodology to produce the C-B bond is poised to support a myriad of subsequent transformations. These transformations include Suzuki couplings, aminations, oxidations, halogenations, cyanations, and trifluoromethylations.Typical iridium catalyzed CHBs proceed through an iridium trisboryl with a bidentate ligand such as bipyridine or 1,10-phenanthroline. The selectivity of these standard catalysts is generally driven by sterics
일반주제명Organic chemistry.
Chemistry.
언어영어
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